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Introduction

So you want to learn more about segmented gamma scanning.

Let's first recap what you should already know – and if you're unsure about this, feel free to check out the beginner course again.

Objectives of Segmented Gamma Scanning

The aim is to identify the gamma-emitting nuclides contained within a confined object (e.g., a 200 L drum) and, if possible, quantify them as well. For this, a suitable detector system is used to measure the gamma radiation emitted from the object, more specifically the gamma spectrum. The detector system can be moved around the object with a mechanical device. This allows for the determination of the distribution of gamma radiation emitted from the surface of the object for each radionuclide and visualized as spatial distributions (OVTs).

From the peak areas of the radionuclides identified in the summed spectrum, which are converted into count rates, and a suitable evaluation model, the activities of the respective radionuclides can be calculated.

Note:
Since this measurement method can only identify radionuclides whose emitted (gamma) radiation can also be measured outside the object, it cannot be assumed based solely on these results that there are no additional radioactive substances contained within the studied object.

Measurement Methods

There are two measurement methods: open geometry and collimated geometry. In both cases, a suitable detector system is used in conjunction with a collimator that limits the area from which radiation can fall onto the detector.

In the measurement in open geometry, collimation is done based on the object dimensions. The collimator here serves only to shield from gamma radiation that is not coming from the object, i.e., from the environment. The detector therefore “sees” only the object. An improvement of the data reliability is achieved when the object is rotated during measurement, allowing the detector to “see” the object from all sides.

Schematic representation of the measurement method in collimated geometry. The detector (right) sees a part of the entire object. The detection cone (gray), which determines the field of view, is determined by a suitable collimator (left in front of the detector). By scanning with an appropriate mechanical device, the entire surface of the object is captured.

Schematic representation of the measurement method in open geometry. The detector (right) sees the entire object (left). The detection cone (gray), which defines the field of view, is determined by a suitable collimator.

In collimated geometry, the collimator limits the field of view to a small section of the object. Through scanning of the entire surface of the object, it can be determined where gamma radiation emerges from the object's surface. This requires a mechanical device that allows for the corresponding positioning of the detector and the object relative to each other.

Schematic representation of the measurement method in collimated geometry. The detector (right) sees a section of the entire object. The detection cone (gray), which defines the field of view, is determined by a suitable collimator (left in front of the detector). By scanning with an appropriate mechanical device, the entire surface of the object is captured.

Schematic representation of the measurement method in collimated geometry. The detector (right) sees a section of the entire object. The detection cone (gray), which defines the field of view, is determined by a suitable collimator (left in front of the detector). By scanning with an appropriate mechanical device, the entire surface of the object is captured.

Summary

Segmented gamma scanning (often abbreviated as SGS) refers to a special method of obtaining measurement data using gamma spectrometry. The method is usually applied to large volume objects containing radioactive content, such as 200 L waste containers. With the help of the measurement data, the (gamma-emitting) radioactive nuclides contained in the object can be identified, and their activities and nuclide masses can be determined with suitable evaluation procedures. In the measurement, the surface of the object is scanned with a suitable collimated detector, the gamma spectrum is measured for each position, and stored. The detector, collimator, and mechanical device that controls the movement of the object and/or the collimated detector are referred to as a segmented gamma scanner.

Photo of a typical segmented gamma scanner with an electro-cooled HPGe detector measuring a 200 L waste container.

Photo of a typical segmented gamma scanner with an electro-cooled HPGe detector measuring a 200 L waste container

The gamma spectra stored for each measurement position can be summed to create a summed spectrum, from which the radionuclides contained within the object can be determined based on their characteristic lines. Additionally, the net peak area of a characteristic line of a radionuclide can be determined for each measured position and visualized in a false color representation on a diagram whose axes correspond to the movement of the measurement.

Spatial distribution for the 59 keV line of nuclide 241Am in a completely filled 200 L drum. The measurement was conducted in multi-rotation mode (73 height and 24 angle positions).

Spatial distribution for the 911 keV line of nuclide 228Ac in a completely filled 200 L drum. The measurement was conducted in multi-rotation mode (73 height and 24 angle positions).

Spatial distribution for the 911 keV line of nuclide 228Ac in a completely filled 200 L drum. The measurement was conducted in multi-rotation mode (73 height and 24 angle positions).

The two images show the resulting spatial distributions from a multi-rotation scan on a 200 L waste container for the two nuclides 241Am and 228Ac. The horizontal positions represent the angle positions, and vertically the height position of the container. From the two images, it is immediately obvious that the activities in the containers are not homogeneously distributed and are located at different positions within the container.

From the spatial distribution for 241Am, it is also evident that the container is likely filled to the top since the radionuclide is detected just below the maximum possible fill height of the container at 760 mm. Additionally, the spatial distributions indicate that the two radionuclides are confined to very small volumes within the waste matrix. For 241Am, it could potentially be two sources or a single source with a (narrow) absorbing part between the source and the detector at a rotation angle of approximately 60°.

Many other insights can similarly be derived from the spatial distributions of the various detected radionuclides and their characteristic lines.

Are you ready?

With the following questions, you can determine whether you already possess sufficient knowledge for the section “Advanced” to make the most of this section. If you cannot answer the questions correctly or feel unsure, we recommend first reading the beginner course on the topic of segmented gamma scanning. However, you can also skip the questions and start directly with the first topic of the advanced course, which is the construction of a segmented gamma scanner. By answering the last question, you will also be redirected to this page.

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Contact

Dr. Thomas Bücherl
Technische Universität München
Radiochemie München RCM
Walther-Meißner-Str. 3
85748 Garching
Deutschland

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